Abstract: The disclosed method and handheld analyzer of elemental concentration measurement is based on spectral analysis of high temperature highly ionized plasma generated by laser-generated pulses. Due to a high pulse energy and short pulse duration, high intensity singly and multiply charged ion lines in addition to neutral atomic lines are excited. The pulsed laser source of the disclosed analyzer is configured to output a train of pulses of signal light at a 1.5-1.6 signal wavelength at a pulse repetition rate from 0.1 to 50 kHz, pulses duration from 0.01 to 1.5 ns, pulse energy between 100 and 1000 uJ and has a beam spot on the surface of the sample varying 1 to 60 ?m. The above-described parameters provide at least a 20 GW/cm2 laser power density sufficient to induce a high temperature, highly ionized plasma (plasma) which allows measuring the carbon concentration in carbon steels by employing doubly charged ionic line CII with a detection limit down to 0.