Abstract: The present invention is directed to a method for enhancing biogenic methanogenesis in carbon-containing materials. The process includes evaluating existing geophysical conditions in a site, identifying optimal geophysical conditions for biogenic methanogenesis, introducing an enhancing fluid into the site configured to alter the existing geophysical conditions, assessing the altered geophysical conditions, comparing the altered geophysical conditions to the optimal geophysical conditions, and repeating the evaluating, introducing, assessing, and comparing steps until the altered geophysical conditions more closely resemble the optimal geophysical conditions. The enhancing fluid contains microorganisms, chemicals, and/or nutrients.