Abstract: A fractal microstructure which includes multi-walled carbon nanotubes suited for customizable volumetric energy and power densities. Electrode monoliths can be formed from a variety of process steps including some or all of RF polymerization, RF coalescence and ripening at intersections, and multi-walled carbon nanotube crosslinking. The resulting nanocomposite is capable of performing all five functions of an electrode while at the same time offering robust mechanical strength and significantly improved energy storage capabilities through, among other things, intra- and inter-particle interlocking.