Abstract: An actinium-227 production device having a plurality of metallic or ceramic caplets, each enclosing a radium-226 compound in redundantly nested sealed cylinders. The radium-226 compound is compacted into a disk and diluted with heat transporting ceramic materials. A thermal neutron shield including spectrum shaping materials to protect actinium-227 produced from exposure to thermal neutrons is included along with a strong neutron absorber to shape the neutron spectrum such that radium-226 nuclei are exposed to neutrons in the higher epithermal energy groups upon entry into the target with an energy of between 20 eV and 1 KeV.

Abstract: A neutron generator and isotope production apparatus and method of using the same to produce commercially and medically useful neutrons. The gamma,n reaction produces neutrons in beryllium and deuterium and the spectrum of the neutrons generated is shaped to optimize capture of the neutrons in a gamma emitting isotope. The gammas interact with target materials to produce large quantities of neutrons.

Abstract: A large enhancement of neutron flux is realized when a primary target of D2O and H2O is contained in a vessel, is irradiated by an electron beam incident on a gamma converter and where the vessel is enclosed within a neutron reflector material including Nickel and Polyethylene. A very large enhancement of neutron flux is realized when a secondary target of LEU is mixed with the primary target resulting in a very large enhanced production of Molybdenum-99. The primary target and the secondary target is contained in cylindrical or spherical vessels.

Abstract: This disclosure concerns a new method for preparing radioisotopes, such as molybdenum-99, by alpha particle irradiation, such as by alpha particle irradiation of zirconium-96. Molybdenum-99 is a precursor to the medically-significant radioisotope technetium-99m. Also disclosed are novel compositions containing one or more of technetium-99m, molybdenum-99 and zirconium species. Systems for producing molybdenum-99 and technetium-99m, including alpha particle generators and irradiation targets, also are described.

Abstract: A neutron generator and isotope production apparatus and method of using the same to produce commercially and medically useful neutrons. The gamma,n reaction produces neutrons in beryllium and deuterium and the spectrum of the neutrons generated is shaped to optimize capture of the neutrons in a gamma emitting isotope. The gammas interact with target materials to produce large quantities of neutrons.

Abstract: A large enhancement of neutron flux is realized when a primary target of D2O and H2O is contained in a vessel, is irradiated by an electron beam incident on a gamma converter and where the vessel is enclosed within a neutron reflector material including Nickel and Polyethylene. A very large enhancement of neutron flux is realized when a secondary target of LEU is mixed with the primary target resulting in a very large enhanced production of Molybdenum-99.

Abstract: At least one very long lived isotope, such as I-129, and a moderator, such as MgH2, is ground, homogeneously mixed and contained in a target assembly which can be at least one target assembly capable of being accessed and vented. The homogeneous mixture is a target which is irradiated, preferrably by a fast reactor flux, thereby transmuting the at least one isotope to a stable or short lived isotope. Resulting gasses, short lived and stable isotopes have medical and industrial uses and value. The transmuted short lived or stable isotopes do not require long term storage.

Abstract: A neutron generator and method of using the same to produce commercial and medical isotopes. Isotopes are transmuted using fission spectrum neutrons produced in neutron multiplier alloys proximate a target isotope. The produced neutron fission spectrum is tailored or shaped by alloys disposed between the multiplier alloys and the target isotope. The tailoring alloys selectively convert the neutron fission spectrum to a nearly coherent distribution of selected high energy, fast, epithermal, or thermal neutrons. The tailoring alloys are engineered to slow the fission spectrum neutrons to the resonance energies of the selected target isotopes through scattering or hydriding of selected components of high temperature aluminum alloys that optimize neutron capture in engineered target alloys.

Abstract: This disclosure concerns a new method for preparing radioisotopes, such as molybdenum-99, by alpha particle irradiation, such as by alpha particle irradiation of zirconium-96. Molybdenum-99 is a precursor to the medically-significant radioisotope technetium-99m. Also disclosed are novel compositions containing one or more of technetium-99m, molybdenum-99 and zirconium species. Systems for producing molybdenum-99 and technetium-99m, including alpha particle generators and irradiation targets, also are described.

Abstract: A solid tag material which generates stable detectable, identifiable, and measurable isotopic gases on exposure to a neutron flux to be placed in a nuclear reactor component, particularly a fuel element, in order to identify the reactor component in event of its failure. Several tag materials consisting of salts which generate a multiplicity of gaseous isotopes in predetermined ratios are used to identify different reactor components.

Abstract: A method of detecting the failure of a sealed non-fueled core component of a liquid-metal cooled fast reactor having an inert cover gas. A gas mixture is incorporated in the component which includes Xenon-124; under neutron irradiation, Xenon-124 is converted to radioactive Xenon-125. The cover gas is scanned by a radiation detector. The occurrence of 188 Kev gamma radiation and/or other identifying gamma radiation-energy level indicates the presence of Xenon-125 and therefore leakage of a component. Similarly, Xe-126, which transmutes to Xe-127 and Kr-84, which produces Kr-85.sup.m can be used for detection of leakage. Different components are charged with mixtures including different ratios of isotopes other than Xenon-124. On detection of the identifying radiation, the cover gas is subjected to mass spectroscopic analysis to locate the leaking component.