Abstract: There have been cases where transistors formed using oxide semiconductors are inferior in reliability to transistors formed using amorphous silicon. Thus, in the present invention, a semiconductor device including a highly reliable transistor formed using an oxide semiconductor is manufactured. An oxide semiconductor film is deposited by a sputtering method, using a sputtering target including an oxide semiconductor having crystallinity, and in which the direction of the c-axis of a crystal is parallel to a normal vector of the top surface of the oxide semiconductor. The target is formed by mixing raw materials so that its composition ratio can obtain a crystal structure.

Abstract: A halogenated flame retardant for a thermoplastic resin with carbonyl linkages in the main chain such as polyethylene terephthalate or polybutylene terephthalate is obtained by the modification of a brominated bisphenol A epoxy resin optionally advanced with brominated bisphenol A by reaction of the epoxy groups with a C1-C8 alcohol such as methanol or butanol to the extent that the ratio of unmodified epoxy groups to alcohol-modified epoxy groups is from 2/1 to 1/2.

Abstract: A halogen containing fire retardant represented by chemical formula (1) wherein the end groups X and Y are composed by A or B represented by chemical formula (2); and the said fire retardant is a mixture of the composition containing 1 to 40% of X=Y=A, 30 to 70% of X=A and Y=B, smaller than 70% of X=Y=B and, degree of polymerization n is n.gtoreq.0 wherein the content of n=0 is smaller than 60% to the total amount. ##STR1## wherein A and B are represented by following chemical formulae, and R of chemical formula B is an alkyl group of carbon number 1 to 8 alone, or 1 to 79% of alkyl group of carbon number 1 to 8 and 79 to 1% of tribromophenyl group, and total amount of R is smaller than 80%.

Abstract: A fire-retardant compound including bromine indicated by general formula (1), wherein the end group X and Y are comprised by A or B shown in formula (2), and the said fire-retardant compound is a mixture of the composition including 15 to 30% of X=Y=A, the composition including 40 to 60% of X=A and Y=B and the composition including 20 to 35% of X=Y=B, and degree of polymerization n is indicated by an integral number from 0 to 30, and a flame-retarded thermoplastic resin including said fire-retardant compound.

Abstract: A fumigation apparatus is provided which uses mixed gas of hydrogen phosphide and methyl bromide, said mixed gas containing hydrogen phosphide at a high concentration, and which is free from the risk of ignition and safe. The apparatus, furthermore, is capable of fumigation that can completely kill noxious insects infesting green plants within a short time, exhibiting very little phytotoxicity on the plants and leaving extremely little residual fumigating agent after fumigation. Said apparatus is composed of (a) a system for purging air and hydrogen phosphide in a hydrogen phosphide path; (b) a system for hydrogen phosphide supply and transfer from a hydrogen phosphide bomb to a mixer through a humidifier; (c) a system for methyl bromide supply and transfer from a methyl bromide bomb to the mixer; and (d) a system for transferring the mixed gas from the mixer to a fumigation chamber.

Abstract: An improved method of fumigating fresh plants on which pests are parasitic. The method comprises maintaining the fresh plants in a gaseous atmosphere composed of 10 to 50 mg/liter of methyl bromide, 0.01 to 10 mg/liter of hydrogen phosphide, and 1 to 50% by volume of carbon dioxide. The method can surely kill the pests on the plants without causing phytotoxicity.