Abstract: An aerial sampler system includes an enclosure, a transfer system, and a measurement system. The enclosure is connected to an external surface of an aerial vehicle and receives atmospheric flow from the external surface of the aerial vehicle. The enclosure also directs at least some of the atmospheric flow into an aperture in the external surface. The transfer system transfers some of the atmospheric flow from the aperture to a measurement system. The measurement system is internal to the external surface of the aerial vehicle and measures atmospheric trace gases in the atmospheric flow.