Abstract: Systems and methods are provided for depositing a structured paint material on a surface. According to one embodiment, the method comprises introducing an initiator to a paint composition comprising methyl methacrylate (MMA) and a first retroreflective element to produce a liquid mixture, depositing the liquid mixture on a surface of a substrate to produce a layer of structured paint material, and depositing a layer of a second retroreflective element onto at least a portion of an upper surface of the deposited layer of structured paint material, and wherein a coefficient of retroreflected luminance of the layer of structured paint material is at least 1400 mcd/m2/lux.