Abstract: A method for preparing carbon-functionalized praseodymium oxide includes the following steps: dissolving Pr(NO3)3·6H2O in an acid dye solution and stirring to form a mixed solution; adding NH3H2O dropwise in the mixed solution while stirring to adjust a pH value of the mixed solution, thereby forming a suspension, and then aging the suspension for 2 to 4 hours; filtering, washing with water, washing with alcohol, and drying the aged suspension to obtain a carbon-functionalized Pr6O11 precursor; and placing the carbon-functionalized Pr6O11 precursor in a tube furnace under a protection of nitrogen, heating the carbon-functionalized Pr6O11 precursor to a sintering temperature at a heating rate of 4 to 6 degrees Celsius/min, keeping at the sintering temperature for 3 to 4 hours, and then cooling to room temperature, thereby obtaining the carbon-functionalized Pr6O11.