Abstract: A method of making molded parts employing Shape Deposition Manufacturing (SDM) techniques. First, SDM processes are used to make a layered structure having support segments and mold segments. The support segments are made of material which may be removed from the mold segments (e.g. dissolved or melted). The mold segments are made of a material which can function as a mold. The mold and support segments are sequentially deposited (e.g. in layers) and shaped (e.g. machined) to form a mold. The support segments define the shape of the part to be manufactured. The mold segments are removed from the support segments by dissolving or melting away the support segments, leaving an empty mold. Then, part material is cast into the empty mold. The mold is removed, providing a molded part. The part material can be a gelcasting slurry, for example. The present method provides homogeneous or heterogeneous parts having shapes which are accurately defined by the SDM process.