Abstract: The present disclosure provides a temporally-resolved and spatially-resolved pump-probe control system and a method. The system includes an ultrafast femtosecond laser device, an optical parametric oscillator, a displacement delay module, a micro-drive rotation module, an objective lens, a sample stage, a coupled photoelectric amplifier and a computer terminal. The control system of the present disclosure integrates a temporally-resolved pump-probe function and a temporally-resolved and spatially-resolved pump-probe function. The present disclosure can realize pump-probe temporally-resolved scanning, one-dimensional temporally-resolved and spatially-resolved scanning, and two-dimensional temporally-resolved and spatially-resolved scanning under full-automatic control, and real-time data is visualized and synchronously written into batch files.