Abstract: A novel nickel-carbon electrode, and methods for making the same, have been developed. The nickel-carbon electrode comprises an active mass (e.g., a nickel oxyhydroxide, hydroxide or oxide) deposited to a carbon foam using any one of chemical deposition, thermal deposition or electrochemical deposition. The nickel-carbon electrode is formed or “activated” through a series of charge-discharge cycles. The nickel-carbon electrode is comparable in volumetric capacities (mAh/cc) with commercial nickel electrodes but higher in gravimetric capacities (mAh/g). The nickel-carbon electrode may be used in rechargeable nickel-based batteries which have applications in cordless appliances, portable devices, standby power systems, the aerospace industry, and hybrid electric vehicles.