Abstract: The present invention relates to a chemical looping combustion and carbon dioxide direct reduction (CLC-CDR) integration system and an operation method thereof, particularly to a chemical looping combustion and carbon dioxide direct reduction (CLC-CDR) integration system including: an air reactor, wherein an oxygen carrier particle is oxidized by reacting with injected air and air from which oxygen was partially removed is discharged; a fuel reactor, wherein the oxidized oxygen carrier particle is supplied, a supplied fuel is reacted to reduce the oxidized oxygen carrier particle, and carbon dioxide including H2O is discharged; and a carbon dioxide reduction reactor, wherein the reduced oxygen carrier particle is supplied, supplied carbon dioxide is reacted to discharge carbon monoxide, and the reduced oxygen carrier particle is partially oxidized and supplied to the air reactor.