Abstract: Methods of forming a gate structure for an integrated circuit memory device include forming a metal oxide dielectric layer on an integrated circuit substrate. Ions of a selected element from group 4 of the periodic table and having a thermal diffusivity of less than about 0.5 centimeters per second (cm2/s) are injected into the dielectric layer to form a charge storing region in the dielectric layer with a tunnel dielectric layer under the charge storing region and a capping dielectric layer above the charge storing region. The substrate including the metal oxide dielectric layer is thermally treated to form a plurality of discrete charge storing nano crystals in the charge storing region. A gate electrode layer is formed on the dielectric layer.