Abstract: A process for recovering uranium and/or thorium from a liquid containing uranium and/or thorium is disclosed, which comprises making a precipitate composed mainly of amorphous silica formed by adding water glass to the liquid containing uranium and/or thorium, capturing the uranium and/or thorium in the liquid by the precipitate, treating the precipitate with acid to elute the captured uranium and/or thorium, adding ammonia or hydrogen peroxide to an acidic solution containing the eluted uranium and/or thorium to form a precipitate composed of ammonium salt or peroxide of the uranium and/or thorium, and filtering out the ammonium salt or peroxide precipitate. Thus, high purity solid uranium and/or thorium reutilizable for manufacture of nuclear fuel material can be recovered in high yield.