Abstract: Magnetostrictive particulate composites with a preferred crystal orientation of the particles and methods for their manufacture are described. In a representative embodiment, a 25% volume Terfenol-D fraction polymer matrix composite was fabricated in a magnetic field using geometric anisotropy to orient needle shaped particles with long axis [112] orientation along the length of the composite. Results demonstrate that the magnetostriction of a [112] oriented particle composite saturates near 1600 ppm. This is a significant increase when compared to composites without preferential orientation (1200 ppm) and represents the largest reported magnetostriction for a particulate composite material.