Abstract: An operation control method is provided. The method is applied on an operation control system. The system includes an operation device and an electronic device. The operation device includes an infrared emitter to emit infrared rays. The electronic device includes a display unit and infrared receivers. The infrared ray creates a light/heat spot on the display unit. Infrared receivers receive the infrared ray emitted by the infrared emitter. The infrared receiver receiving one infrared ray generates a corresponding signal. The method includes receiving the signal generated by the infrared receiver, determining which infrared receivers generated the signal to determine the light spot on the display unit, and controlling the electronic device to execute the corresponding function according to signals created by the light spot or spots striking the display unit.