Abstract: A process for preparing dicalcium silicate includes providing a starting material comprising calcium carbonate (CaCO3) and silicon dioxide (SiO2), wherein a molar ratio of calcium:silicon (C:S) is from 1.5:1 to 2.5:1. At least one of an inorganic alkali metal salt and an alkaline earth metal salt is added as a mineralizing agent to the starting material in an amount of from 0.5 wt.-% to 20 wt.-%, based on a total weight of the starting material. The starting material is reacted with the mineralizing agent in a gas atmosphere having a CO2 partial pressure of from 0.05 MPa to 0.2 MPa at a temperature of from 900° C. to 1100° C. so as to obtain a dicalcium silicate product. The dicalcium silicate product comprises a content of an unreacted starting material of <5 wt.-% and a total carbon content of <1.5 wt.-%, each based on a weight of the dicalcium silicate product.