Abstract: Herein, a polymer-based device capable of lifting many times its own mass was fabricated by drying a solution of the polycation poly (diallyldimethyl ammonium chloride) (pDADMAC) on a surface coated with charged poly (N-isopropylacrylamide)-based microgels. Due to strong polymer-polymer and polymer-surface interactions, when the pDADMAC solution dries on the microgel-modified surface, it bends. If the surface is flexible, it curls up into a scroll like structure, that can be opened up at high (ca. 80%) humidity. This process is fully reversible, i.e., if the humidity is decreased, the surface curls back up. This expansion/contraction behavior is capable of lifting relatively large masses, many times its own mass, and can potentially be used as an artificial muscle.

Abstract: Herein, a polymer-based device capable of lifting many times its own mass was fabricated by drying a solution of the polycation poly (diallyldimethyl ammonium chloride) (pDADMAC) on a surface coated with charged poly (N-isopropylacrylamide)-based microgels. Due to strong polymer-polymer and polymer-surface interactions, when the pDADMAC solution dries on the microgel-modified surface, it bends. If the surface is flexible, it curls up into a scroll like structure, that can be opened up at high (ca. 80%) humidity. This process is fully reversible, i.e., if the humidity is decreased, the surface curls back up. This expansion/contraction behavior is capable of lifting relatively large masses, many times its own mass, and can potentially be used as an artificial muscle.