Abstract: A composition to immobilize nuclear containing waste comprising at least one radioactive element or alloy of uranium, graphite, magnesium, and aluminum, and a method of using the same to immobilize the nuclear containing waste into a solid wasteform. The composition comprises at least one mineral phase forming element or compound for reacting with the at least one radioactive element or alloy. The composition further comprises at least one glass-forming element or compound to form a glass phase that will incorporate waste radioisotopes and impurities that do not react with the mineral phase forming element or compound.

Abstract: A composition to immobilize nuclear containing waste containing at least one radioactive element or alloy of uranium, graphite, magnesium, and aluminum is disclosed. The composition comprises at least one mineral phase forming element or compound for reacting with the at least one radioactive element or alloy. The composition further comprises at least one glass-forming element or compound to form a glass phase that will incorporate waste radioisotopes and impurities that do not react with the mineral phase forming element or compound. A method of using the disclosed composition to immobilize the nuclear containing waste into a solid wasteform is also disclosed.