Abstract: An ultrasonic-rotary composite atomization mechanism comprises a housing and an ultrasonic unit passing through the housing and free to rotate with respect to the housing. A dynamic unit is installed in a position of the ultrasonic unit, which is corresponding to the housing, to drive the ultrasonic unit to rotate with respect to the housing. The ultrasonic unit includes a material supply channel, a vibration member disposed in the ultrasonic unit, and a vibration-rotation cup connected with the material supply channel. The material supply channel carries a liquid into the vibration-rotation cup. The dynamic unit and vibration member operate simultaneously to make the vibration-rotation cup rotate at high speed and vibrate ultrasonically. Thus is generated a synergistic effect: the ultrasonic vibration uses inertia force to break the cohesion and disperse the liquid, and the high-speed rotation generates centrifugal force to atomize the liquid.