Abstract: A Fe—Ni compound oxide is used as an oxygen carrier for chemical looping combustion process, wherein the structure of the Fe—Ni compound oxide is a single-phase spinel structure. The method for manufacturing the Fe—Ni compound oxide of the invention includes the following steps: mixing Fe2O3 and NiO to obtain a mixing solution and ball milling the mixing solution by the solid state ball milling method; drying the mixing solution to obtain a precipitate; granulating the precipitate and then calcining the granulated precipitate to obtain the Fe—Ni compound oxide. Accordingly, the Fe—Ni compound oxide manufactured by the method of the invention is provided with high oxidation rate and high reduction rate, and capable of keeping loops and producing hydrogen gas.

Abstract: A chemical looping combustion method using a dual metal compound oxide includes the following steps: a fuel material combusting with the dual metal compound oxide in a first reactor to obtain a metal product; supplying the metal product obtained in the first reactor into a second reactor, and the metal product reacting with the air in the second reactor to obtain the dual metal compound oxide; and, supplying the dual metal compound oxide obtained in the second reactor into the first reactor. The dual metal compound oxide used in the chemical looping combustion process has high oxidation rate as well as high reduction rate so as to increase the efficiency of the chemical looping combustion process.