Abstract: Disclosed is a large-angle LED lens including a main body which has an incident surface on the inner side of the main body and an exit surface on the outer side thereof. The surfaces are provided symmetrically about the central axis of the main body. The incident and exit surfaces are transparent concave and convex surfaces, respectively. The maximum thickness d1 of the main body at the lower part and the minimum thickness d2 thereof at the top satisfy the relation: 4<d1/d2<6; the concave depth h1 of the concave surface and the thickness d2 satisfy the relation: h1>4*d2; and the convex height h2 of the convex surface and the thickness d2 satisfy the relation: h2>5*d2. With the disclosure, the light-emitting angle is increased while maximizing the utilization of the light. A large-angle emission LED light source module is also disclosed herein.