Abstract: The present invention relates to a manufacturing method of granulated complex molecular sieve composition having multifunction and useful for removal agent of harmful gas of cigarette or treatment agent of water purification etc. as having multifunctioned adsorption capacity and excellent anti-abrasion property, and convenient process, in particular, to a manufacturing method which is comprised of granulating by mixing alkali metal silicate aqueous solution to mixture of zeolites of various types and active carbon and treating it with water solution of alkali earth metal salt without calcination, and drying.