Abstract: The invention describes a general method of controlling and/or substantially eliminating weeds by applying compositions comprising chloride ion-containing compounds having chloride concentrations that effectively control the growth of and/or substantially eliminate weedy species such as bermudagrass and other grassy and broadleaved weeds, without harming salt-tolerant grasses such as Seashore paspalum or the environment. The compositions may also include chelants or other additives that enhance movement of the composition into the weedy species shoots and other grass components for control as well as other chemicals or compounds applied prior to or after application of the compositions to control and eliminate weedy species. The methods of the invention are particularly useful in developing, managing and maintaining golf courses, vegetative or seed production fields, sports fields, lawns, landscapes and any other paspalum plantings (e.g., forages, land stabilization, bioremediation).