Abstract: The present invention provides compositions and nanomaterials comprising a metal based high entropy oxide comprising at least five metals and their oxides distributed in a crystal structure, with high configurational entropy, a high number of oxygen vacancies and active catalytic sites. The present invention also relates to methods of synthesis of said compositions and nanomaterials using microwave irradiation and methods of use of said compositions and nanomaterials in analyte sensing as nanozymes, electrochemical sensors, and colorimetric sensors.

Abstract: An epidermal microfluidic device includes a rigid substrate defining microfluidic features (e.g., portions of channels, valves within channels, and/or portions of reservoirs) with gradient variation in height thereof. A rigid substrate of such a devices may permit flexure during use without breakage and without distortion of microfluidic features therein, such as by providing channel-defining, reduced-width linking portions extending outward between a central portion and reservoir portions, with the reservoir portions lacking direct coupling therebetween. An epidermal interface layer comprising a flexible material and defining a first aperture may be adhered to skin of a user, and multiple microfluidic devices may be sequentially provided over, and removed from, the epidermal interface layer to collect multiple independent, pristine sweat samples during an extended active collection period.

Abstract: An aspect of the present disclosure provides a system for aerosol jet printing an aerosolized particle source configured to selectively provide aerosolized particles, a nozzle configured to deposit aerosolized particles on a substrate, an actuator configured to generate acoustic energy for migrating the particles, and a generator configured to selectively energize the actuator. The nozzle includes a proximal inlet configured for passage of aerosolized particles, a column configured to focus the aerosolized particles when vibrated by an actuator, and a distal opening configured for deposition of the particles on a substrate.

Abstract: A method of three-dimensional (3D) printing includes applying a solution to a channel. The solution includes a plurality of anisotropic particles suspending in the solution. Acoustic waves are applied to the channel. The frequency of the acoustic waves is configured to organize the plurality of anisotropic particles into one or more columns of organized anisotropic particles. The channel is connected to a printhead and a waste outlet. The solution comprising the one or more columns of organized anisotropic particles is deposited on a substrate via the printhead outlet.

Abstract: A method of three-dimensional (3D) printing includes applying a solution to a channel. The solution includes a plurality of anisotropic particles suspending in the solution. Acoustic waves are applied to the channel. The frequency of the acoustic waves is configured to organize the plurality of anisotropic particles into one or more columns of organized anisotropic particles. The channel is connected to a printhead and a waste outlet. The solution comprising the one or more columns of organized anisotropic particles is deposited on a substrate via the printhead outlet.

Abstract: A three-dimensional (3D) printer includes an acoustophoresis device having at least a first inlet, a first outlet, and a channel defined between the first inlet and the first outlet. A piezoelectric device is adhered to a surface of the acoustophoresis device to generate sound waves within the channel. A printhead is connected to the first outlet of the acoustophoresis device, wherein a solution comprising anisotropic particles is delivered to the at least first inlet and wherein the anisotropic particles are organized into one or more columns along an axis parallel to a direction of flow of the solution by standing acoustic waves generated by the piezoelectric device, wherein the at least one column of anisotropic particles is aligned with the first outlet, and wherein the first outlet is in fluid communication with the printhead to deliver one or more columns of ordered, anisotropic particles to the printhead.

Abstract: An aspect of the present disclosure provides a system for aerosol jet printing an aerosolized particle source configured to selectively provide aerosolized particles, a nozzle configured to deposit aerosolized particles on a substrate, an actuator configured to generate acoustic energy for migrating the particles, and a generator configured to selectively energize the actuator. The nozzle includes a proximal inlet configured for passage of aerosolized particles, a column configured to focus the aerosolized particles when vibrated by an actuator, and a distal opening configured for deposition of the particles on a substrate.

Abstract: Systems and methods for optically measuring displacement of an element include an emitter for emitting an optical signal, a first detector for detecting reflections of the optical signal from the element, a second detector for detecting reflections of the optical signal from a raised cover structure, a processor for receiving the detected reflections from the first and second detectors and removing distortions in the detected reflections from the first detector using the detected reflections from the second detector.

Abstract: A three-dimensional (3D) printer includes an acoustophoresis device having at least a first inlet, a first outlet, and a channel defined between the first inlet and the first outlet. A piezoelectric device is adhered to a surface of the acoustophoresis device to generate sound waves within the channel. A printhead is connected to the first outlet of the acoustophoresis device, wherein a solution comprising anisotropic particles is delivered to the at least first inlet and wherein the anisotropic particles are organized into one or more columns along an axis parallel to a direction of flow of the solution by standing acoustic waves generated by the piezoelectric device, wherein the at least one column of anisotropic particles is aligned with the first outlet, and wherein the first outlet is in fluid communication with the printhead to deliver one or more columns of ordered, anisotropic particles to the printhead.

Abstract: Systems and methods for optically measuring displacement of an element include an emitter for emitting an optical signal, a first detector for detecting reflections of the optical signal from the element, a second detector for detecting reflections of the optical signal from a raised cover structure, a processor for receiving the detected reflections from the first and second detectors and removing distortions in the detected reflections from the first detector using the detected reflections from the second detector.

Abstract: A method of ordering particles suspended in a solution includes providing anisotropic particles suspended in a solution to a channel, wherein the anisotropic particles are unordered when entering the channel. The method further includes applying sound waves to the channel, wherein the frequency of the sound wave is tuned to create one or more columns of particles oriented in the same direction.