Abstract: Embodiments of the present disclosure pertain to compositions comprising particles and a binding material, where the binding material and at least some of the particles are breakably associated with one another to form bound particles. Additional embodiments of the present disclosure pertain to methods of making the compositions by associating particles with a binding material such that the binding material and at least some of the particles become breakably associated with one another to form bound particles. Further embodiments of the present disclosure pertain to methods of additively manufacturing a material on a surface by (a) applying said bound particles onto the surface; (b) breaking at least some of the bound particles into particles; (c) applying an adhesive material onto the surface; and (d) treating the particles and any remaining bound particles to form the additively manufactured material. Additional embodiments pertain to the formed additively manufactured materials.