Abstract: this invention relates to an alloy material for data storage of magneto-optical disk (ADSMO), as well as its manufacturing process. ADSMO is based on manganese, bismuth and doped with aluminum atoms and silicon atoms or by aluminum atoms and boron atoms. The above mentioned elements are deposited onto a transparent substrate in a certain sequence using an evaporation process or sputtering process, and then compact hexagonal cyrstalline structures are formed after being annealed in vacuum. ADSMO has a large magneto-optical Kerr rotation, a small size of crystal grains and a stable structure; its manufacturing process is easy and simple.