Patents by Inventor Yukio Takagi
Yukio Takagi has filed for patents to protect the following inventions. This listing includes patent applications that are pending as well as patents that have already been granted by the United States Patent and Trademark Office (USPTO).
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Patent number: 12239961Abstract: A catalyst, which can be used even under mild conditions and also has durability so as to enable repeated use while maintaining high activity, and with which a reduction reaction for converting an amide compound into an amine compound can be carried out, is provided by means of an amide compound hydrogenation reaction catalyst characterized in that platinum and vanadium are supported on a carrier and a method for producing an amine compound using the same.Type: GrantFiled: March 28, 2018Date of Patent: March 4, 2025Assignees: OSAKA UNIVERSITY, N.E. CHEMCAT CORPORATIONInventors: Kiyotomi Kaneda, Takato Mitsudome, Yukio Takagi
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Patent number: 12187691Abstract: Provided is a catalyst for amide compound hydrogenation characterized in that rhodium and molybdenum are supported on hydroxyapatite, the catalyst for amide compound hydrogenation providing a catalyst that can promote a reduction reaction that converts an amide compound into an amine compound, can be used under moderate conditions, and has durability that allows repeated use thereof while retaining high activity. Also provided is a method for producing an amine compound, the method being characterized by including bringing an amide compound into contact with the catalyst for amide compound hydrogenation to cause hydrogenation, thereby producing an amine compound.Type: GrantFiled: February 20, 2020Date of Patent: January 7, 2025Assignees: Osaka University, N.E. Chemcat CorporationInventors: Kiyotomi Kaneda, Takato Mitsudome, Miho Kimura, Yukio Takagi, Yosuke Imanaka, Hiroyasu Suzuka, Tatsuya Kojima
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Publication number: 20240359169Abstract: The present invention provides an organic metal complex catalyst for an olefin metathesis reaction, which enables the achievement of a higher yield of a desired substance in an olefin metathesis reaction than the conventional catalysts. The organic metal complex catalyst according to the present invention has a structure represented by formula (1) and is used for an olefin metathesis reaction. In formula (1), M represents a coordination center and is an Ru atom or an ion thereof; R1, R2 and R3 may be the same as or different from each other and independently represent a substituent such as a hydrogen atom; R4, R5, R6 and R7 may be the same as or different from one another and independently represent a substituent such as a hydrogen atom; X represents a halogen atom; and R8 represents a substituent having 3 to 20 carbon atoms and having a ? bond.Type: ApplicationFiled: September 16, 2022Publication date: October 31, 2024Applicants: N.E. CHEMCAT CORPORATION, NATIONAL INSTITUTE OF ADVANCED INDUSTRIAL SCIENCE AND TECHNOLOGYInventors: Junchul Choi, Norihisa Fukaya, Kazuhiro Matsumoto, Tomoteru Mizusaki, Yukio Takagi, Yasuhiro Seki
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Patent number: 12110296Abstract: The present invention provides a method for producing a compound represented by formula (2), comprising at least a step of preparing a compound represented by formula (1) and a step of reacting the compound represented by formula (1) with a hydrogen source using a catalyst, wherein R1 and R2 are each independently an alkyl group.Type: GrantFiled: October 7, 2019Date of Patent: October 8, 2024Assignees: N.E. CHEMCAT CORPORATION, OSAKA UNIVERSITYInventors: Kiyotomi Kaneda, Takato Mitsudome, Yoshiyuki Wada, Yukio Takagi
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Patent number: 12017208Abstract: It is an object of the present invention to provide a catalyst for a cross-coupling reaction in which an organometallic complex is sufficiently immobilized on a carrier and an object product can be easily obtained in a high yield and in a relatively short reaction time with a relatively small amount of use. The catalyst for a cross-coupling reaction of the present invention has a carrier part composed of a synthetic resin and an organometallic complex part immobilized on the carrier part by chemical bonding, and has a structure represented by formula (P1), wherein in (P1) R1, R2 may be the same or different, and is a substituent such as a hydrogen atom. R3, R4, R5, R6, R8, R9 may be the same or different and are substituents, such as a hydrogen. X represents a halogen atom, and R7 represents a substituent having 3 to 20 carbon atoms with a ? bond. RS1 represents the main chain of the synthetic resin precursors having —CH2OH group at their end.Type: GrantFiled: August 28, 2019Date of Patent: June 25, 2024Assignees: N.E. CHEMCAT CORPORATION, NATIONAL INSTITUTE OF ADVANCED INDUSTRIAL SCIENCE AND TECHNOLOGYInventors: Tomoteru Mizusaki, Yukio Takagi, Junchul Choi, Norihisa Fukaya, Kazuhiro Matsumoto
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Patent number: 11724249Abstract: Provided are a high-performance Cu—P co-supported zeolite and the like having excellent thermal endurance and catalyst performance. A Cu—P co-supported zeolite comprising at least a small pore size zeolite, and an extra-backbone copper atom and an extra-backbone phosphorus atom supported on the small pore size zeolite, wherein a silica-alumina ratio (SiO2/Al2O3) is 7 or more and 20 or less, a ratio of the copper atom to a T atom (Cu/T) is 0.005 or more and 0.060 or less, a ratio of the phosphorus atom to the T atom (P/T) is 0.005 or more and 0.060 or less, and a ratio of the phosphorus atom to the copper atom (P/Cu) is 0.1 or more and 3 or less.Type: GrantFiled: October 16, 2019Date of Patent: August 15, 2023Assignee: N.E. CHEMCAT CORPORATIONInventors: Yukio Takagi, Kiyohiko Saito, Yasuyuki Banno, Makoto Nagata
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PHOSPHORUS ELEMENT-CONTAINING ZEOLITE AND METHOD FOR PRODUCING PHOSPHORUS ELEMENT-CONTAINING ZEOLITE
Publication number: 20230219822Abstract: A small-pore zeolite that is modified with phosphorus, is excellent in hydrothermal durability, and has an 8-membered oxygen ring structure. The 8-membered oxygen ring structure is CHA, AEI, and AFX. The small-pore zeolite incudes at least an aluminum element, a silica element, a phosphorus element, wherein the phosphorus element is defined by expression (1), and the small-pore zeolite has an 8-membered oxygen ring structure being of CHA, AEI, or AFX. The phosphorus element that modifies the zeolite is unevenly distributed and richly contained on the surface layer side of the zeolite. A method for producing a phosphorus element-containing zeolite.Type: ApplicationFiled: April 6, 2021Publication date: July 13, 2023Applicant: N.E. CHEMCAT CORPORATIONInventors: Yukio TAKAGI, Yasuyuki BANNO, Kiyohiko SAITO, Hiroyasu SUZUKA, Yosuke IMANAKA, Takahiko ISHIKAWA -
Publication number: 20220213110Abstract: The present invention provides, for example, a compound represented by formula (1), or a salt thereof: wherein R1 to R4 are each independently an alkyl group.Type: ApplicationFiled: May 8, 2020Publication date: July 7, 2022Applicants: OSAKA UNIVERSITY, N.E. CHEMCAT CorporationInventors: Takato MITSUDOME, Yukio TAKAGI, Kiyohiko SAITO, Hiroyasu SUZUKA, Yosuke IMANAKA, Yasuyuki BANNO
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Publication number: 20220144789Abstract: Provided is a catalyst for amide compound hydrogenation characterized in that rhodium and molybdenum are supported on hydroxyapatite, the catalyst for amide compound hydrogenation providing a catalyst that can promote a reduction reaction that converts an amide compound into an amine compound, can be used under moderate conditions, and has durability that allows repeated use thereof while retaining high activity. Also provided is a method for producing an amine compound, the method being characterized by including bringing an amide compound into contact with the catalyst for amide compound hydrogenation to cause hydrogenation, thereby producing an amine compound.Type: ApplicationFiled: February 20, 2020Publication date: May 12, 2022Applicants: OSAKA UNIVERSITY, N.E. CHEMCAT CORPORATIONInventors: Kiyotomi KANEDA, Takato MITSUDOME, Miho KIMURA, Yukio TAKAGI, Yosuke IMANAKA, Hiroyasu SUZUKA, Tatsuya KOJIMA
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Publication number: 20220111367Abstract: Provided is a hydrogenation catalyst for an amide compound, containing hydroxyapatite and platinum and vanadium that are fixed on the hydroxyapatite, 15 to 80% of the surface of the platinum being covered with vanadium. The hydrogenation catalyst can promote a reduction reaction in which an amide compound is converted into an amine compound, can be used under mild conditions, and has such durability that the catalyst can be repeatedly used while retaining a high activity.Type: ApplicationFiled: August 30, 2019Publication date: April 14, 2022Applicants: OSAKA UNIVERSITY, N.E. CHEMCAT CORPORATIONInventors: Kiyotomi KANEDA, Takato MITSUDOME, Miho KIMURA, Yukio TAKAGI, Yoshiyuki WADA
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Publication number: 20220032278Abstract: An organometallic complex catalyst that makes it possible to obtain a higher yield of a desired product than conventional catalysts in a cross-coupling reaction. The organometallic complex catalyst has a structure represented by formula (1) and is for use in a cross-coupling reaction. In formula (1), M is the coordination center and represents a metal atom such as Pd or an ion thereof. R1, R2, and R3 may be the same or different and are a substituent such as a hydrogen atom. R4, R5, R6, and R7 may be the same or different and are a substituent such as a hydrogen atom. X represents a halogen atom. R8 represents a substituent that has a ? bond and 3-20 carbon atoms.Type: ApplicationFiled: September 30, 2021Publication date: February 3, 2022Applicants: NATIONAL INSTITUTE OF ADVANCED INDUSTRIAL SCIENCE AND TECHNOLOGY, N.E. CHEMCAT CORPORATIONInventors: Junchul Choi, Norihisa Fukaya, Shunya Onozawa, Kazuhiko Sato, Hiroyuki Yasuda, Tomoteru Mizusaki, Yukio Takagi
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Publication number: 20220008905Abstract: An organometallic complex catalyst is disclosed for use in a cross-coupling reaction. In formula (1), M is the coordination center and represents a metal atom such as Pd or an ion thereof. R1, R2, and R3 may be the same or different and are a substituent such as a hydrogen atom. R4, R5, R6, and R7 may be the same or different and are a substituent such as a hydrogen atom. X represents a halogen atom. R8 represents a substituent that has a n bond and 3-20 carbon atoms. With regard to the electron-donating properties of R1-R7 with respect to the coordination center M of the ligand containing R1-R7 that is indicated in formula (2), R1-R7 are arranged in combination such that the TEP value obtained from infrared spectroscopy shifts toward the high frequency side compared to the TEP value of the ligand of formula (2-1).Type: ApplicationFiled: September 28, 2021Publication date: January 13, 2022Applicants: NATIONAL INSTITUTE OF ADVANCED INDUSTRIAL SCIENCE AND TECHNOLOGY, N.E. CHEMCAT CORPORATIONInventors: Junchul Choi, Norihisa Fukaya, Shunya Onozawa, Kazuhiko Sato, Hiroyuki Yasuda, Tomoteru Mizusaki, Yukio Takagi
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Publication number: 20210380594Abstract: The present invention provides a method for producing a compound represented by formula (2), comprising at least a step of preparing a compound represented by formula (1) and a step of reacting the compound represented by formula (1) with a hydrogen source using a catalyst, wherein R1 and R2 are each independently an alkyl group.Type: ApplicationFiled: October 7, 2019Publication date: December 9, 2021Applicants: N.E. CHEMCAT CORPORATION, OSAKA UNIVERSITYInventors: Kiyotomi KANEDA, Takato MITSUDOME, Yoshiyuki WADA, Yukio TAKAGI
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Publication number: 20210379573Abstract: Provided are a high-performance Cu—P co-supported zeolite and the like having excellent thermal endurance and catalyst performance. A Cu—P co-supported zeolite comprising at least a small pore size zeolite, and an extra-backbone copper atom and an extra-backbone phosphorus atom supported on the small pore size zeolite, wherein a silica-alumina ratio (SiO2/Al2O3) is 7 or more and 20 or less, a ratio of the copper atom to a T atom (Cu/T) is 0.005 or more and 0.060 or less, a ratio of the phosphorus atom to the T atom (P/T) is 0.005 or more and 0.060 or less, and a ratio of the phosphorus atom to the copper atom (P/Cu) is 0.1 or more and 3 or less.Type: ApplicationFiled: October 16, 2019Publication date: December 9, 2021Applicant: N.E. CHEMCAT CORPORATIONInventors: Yukio TAKAGI, Kiyohiko SAITO, Yasuyuki BANNO, Makoto NAGATA
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Patent number: 11167278Abstract: An organometallic complex catalyst that makes it possible to obtain a higher yield of a desired product than conventional catalysts in a cross-coupling reaction. The organometallic complex catalyst has a structure represented by formula (1) and is for use in a cross-coupling reaction. In formula (1), M is the coordination center and represents a metal atom such as Pd or an ion thereof. R1, R2, and R3 may be the same or different and are a substituent such as a hydrogen atom. R4, R5, R6, and R7 may be the same or different and are a substituent such as a hydrogen atom. X represents a halogen atom. R8 represents a substituent that has a ? bond and 3-20 carbon atoms.Type: GrantFiled: December 6, 2017Date of Patent: November 9, 2021Assignees: ADVANCED INDUSTRIAL SCIENCE AND TECHNOLOGY, N.E. CHEMCAT CORPORATIONInventors: Junchul Choi, Norihisa Fukaya, Shunya Onozawa, Kazuhiko Sato, Hiroyuki Yasuda, Tomoteru Mizusaki, Yukio Takagi
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Patent number: 11161103Abstract: An organometallic complex catalyst is disclosed for use in a cross-coupling reaction. In formula (1), M is the coordination center and represents a metal atom such as Pd or an ion thereof. R1, R2, and R3 may be the same or different and are a substituent such as a hydrogen atom. R4, R5, R6, and R7 may be the same or different and are a substituent such as a hydrogen atom. X represents a halogen atom. R8 represents a substituent that has a ? bond and 3-20 carbon atoms. With regard to the electron-donating properties of R1-R7 with respect to the coordination center M of the ligand containing R1-R7 that is indicated in formula (2), R1-R7 are arranged in combination such that the TEP value obtained from infrared spectroscopy shifts toward the high frequency side compared to the TEP value of the ligand of formula (2-1).Type: GrantFiled: December 6, 2017Date of Patent: November 2, 2021Assignees: NATIONAL INSTITUTE OF ADVANCED INDUSTRIAL SCIENCE AND TECHNOLOGY, N.E. CHEMCAT CORPORATIONInventors: Junchul Choi, Norihisa Fukaya, Shunya Onozawa, Kazuhiko Sato, Hiroyuki Yasuda, Tomoteru Mizusaki, Yukio Takagi
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Publication number: 20210308660Abstract: It is an object of the present invention to provide a catalyst for a cross-coupling reaction in which an organometallic complex is sufficiently immobilized on a carrier and an object product can be easily obtained. The catalyst for a cross-coupling reaction of the present invention has a carrier part composed of a synthetic resin and an organometallic complex part immobilized on the carrier part by chemical bonding, and has a structure represented by formula (P1), wherein in (P1) R1, R2 may be the same or different, and is a substituent such as a hydrogen atom. R3, R4, R5, R6, R8, R9 may be the same or different and are substituents, such as a hydrogen. X represents a halogen atom, and R7 represents a substituent having 3 to 20 carbon atoms with a ? bond. RS1 represents the main chain of the synthetic resin precursors having —CH2OH group at their end.Type: ApplicationFiled: August 28, 2019Publication date: October 7, 2021Applicants: N.E. CHEMCAT CORPORATION, NATIONAL INSTITUTE OF ADVANCED INDUSTRIAL SCIENCE AND TECHNOLOGYInventors: Tomoteru Mizusaki, Yukio Takagi, Junchul Choi, Norihisa Fukaya, Kazuhiro Matsumoto
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Patent number: 10882033Abstract: A slurry composition for a catalyst and a method for producing the same, a catalyst and a method for producing the same using the slurry composition for a catalyst. The method omits many heretofore required treatment steps and reduces catalyst production cost. The method comprising the steps of providing a slurry composition for a catalyst, comprising at least an aluminosilicate, Cu, and water, and having a solid concentration of 0.1% by mass to 90% by mass, wherein a component for a catalyst has composition represented by Al2O3·xSiO2·yT2O·zCuO (wherein T is a quaternary ammonium cation, and x, y and z are numbers that satisfy 10?x?40, 0.1?y<2.0, and 0.1?z<2.0, respectively) in terms of molar ratio based on an oxide; coating at least one side of a support with this slurry composition; and heat-treating at 350° C. or higher.Type: GrantFiled: November 21, 2018Date of Patent: January 5, 2021Assignee: N.E. CHEMCAT CORPORATIONInventors: Yukio Takagi, Kiyohiko Saito, Yasuyuki Banno, Makoto Nagata
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Publication number: 20200299239Abstract: An aromatic nitro compound has a structure in which a nitro group and a halogen atom, in a separated state, are directly bonded as substituents to the ring structure of the same ring; a reaction composition is provided which, in a hydrogenation reaction of the nitro group of said aromatic nitro compound, allows selectively hydrogenating the nitro group, and sufficiently reducing the separation of the halogen atom from the ring; also provided is a reaction system that uses this reaction composition. This reaction composition includes a catalyst which, with the aforementioned aromatic nitro compound as reactant, is used in a hydrogenation reaction of at least one of the one or more nitro groups of said reactant. Further, the reaction composition includes a base and an organic solvent. The catalyst includes a carrier, and Fe oxide particles and Pt particles supported by the carrier.Type: ApplicationFiled: February 15, 2017Publication date: September 24, 2020Applicant: N.E. CHEMCAT CORPORATIONInventors: Hiroyasu Suzuka, Tomoteru Mizusaki, Yusuke Nakaya, Yoshiyuki Wada, Yukio Takagi
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Publication number: 20200290024Abstract: Provided is a catalyst mixture which, in a nitro group hydrogenation reaction of an aromatic nitro compound having a structure in which nitro groups and halogen atoms are directly bonded as substituents to a ring skeleton of the same ring while separated from each other, is capable of selectively hydrogenating the nitro groups and sufficiently reducing the removal of the halogen atoms from the ring. This catalyst mixture includes a catalyst which is used in a hydrogenation reaction of at least one among one or more nitro groups present in a reactant, which is an aromatic nitro compound having a structure in which one or more nitro groups and one or more halogen atoms are directly bonded as substituents to a ring skeleton of the same ring while separated from each other. This catalyst mixture further includes a base.Type: ApplicationFiled: February 15, 2017Publication date: September 17, 2020Applicant: N.E. CHEMCAT CORPORATIONInventors: Tomoteru Mizusaki, Hiroyasu Suzuka, Yusuke Nakaya, Yoshiyuki Wada, Yukio Takagi