Abstract: A method of making lithium-ion battery anode comprising step (S1)-step (S3). step (S1): providing a nano-silicon material, and coating a positively charged carbonizable polymer on a surface of the nano-silicon material, to obtain a nano-silicon coated with the positively charged carbonizable polymer. Step (S2): adding CNTs and the nano-silicon coated with the positively charged carbonizable polymer to a solvent; and performing an ultrasonic dispersion to obtain a dispersion. And step (S3): vacuum filtering the dispersion, to obtain a composite film of the CNTs and the nano-silicon coated with positively charged carbonizable polymer.

Abstract: A lithium-ion battery anode is provided. The lithium-ion battery anode comprises a carbon nanotube three-dimensional network structure formed by a plurality of carbon nanotubes intertwined with each other. A plurality of nano-silicon particles coated with amorphous carbon, dispersed in the carbon nanotube three-dimensional network structure, and adhered to surfaces of the plurality of carbon nanotubes. The amorphous carbon is obtained by calcining a positively charged carbonizable polymer. And a carbon nanotube functional layer located on two opposite surfaces of the carbon nanotube three-dimensional network structure, to make the carbon nanotube three-dimensional network structure located between two carbon nanotube functional layers. The carbon nanotube functional layer comprises at least two super-aligned carbon nanotube films stacked and crossed with each other.