Formation Of Plutonium Isotopes Patents (Class 376/182)
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Patent number: 11842823Abstract: A reactor irradiation method is provided that can include irradiating Np or Am spheres within a target assembly of a nuclear reactor to form reacted spheres comprising Pu. The target assembly can define a solid core within an exterior housing, and a void between the exterior housing and the solid core, wherein the spheres occupy at least a portion of the void. The irradiating can include exposing the spheres to a neutron energy spectrum while the spheres are in the void of the target assembly to form irradiated spheres.Type: GrantFiled: June 15, 2020Date of Patent: December 12, 2023Assignee: Battelle Memorial InstituteInventors: Jeffrey A. Katalenich, Bruce D. Reid, Robert O. Gates, Andrew W. Prichard, Bruce E. Schmitt, Jim Livingston
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Patent number: 11075013Abstract: This disclosure describes various configurations and components of a molten fuel fast or thermal nuclear reactor in which one or more primary heat exchangers are located above the reactor core of the nuclear reactor.Type: GrantFiled: November 21, 2019Date of Patent: July 27, 2021Assignee: TerraPower, LLCInventors: Ryan Abbott, Anselmo T. Cisneros, Jr., Mark R. Werner
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Publication number: 20150078504Abstract: In an embodiment, a hybrid molten salt reactor includes a source of energetic neutrons, the energetic neutrons having a typical energy per neutron of 14 MeV or greater, a critical molten salt reactor, and a molten salt comprising a dissolved mixture of fissile actinides and fertile actinides. The molten salt circulates in a loop through the reactor vessel and around the source of energetic neutrons. The fissile actinides and fertile actinides sustain an exothermic nuclear reaction in which the actinides are irradiated by the energetic neutrons, the energetic neutrons inducing subcritical nuclear fission, and undergo critical nuclear fission when circulating through the critical molten salt reactor. A portion of the daughter neutrons generated by nuclear reactions are captured by the fertile actinides in the molten salt and induce transmutation of the fertile actinides into fissile actinides and sustain critical fission chain reactions in the molten salt reactor.Type: ApplicationFiled: April 23, 2014Publication date: March 19, 2015Inventor: Robert Daniel Woolley
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Patent number: 8917807Abstract: A lightly hydrided/deuterated metallic plutonium-thorium fuel for use in a fast fission pool-type nuclear reactor cooled with liquid metal coolants, including lithium-7 lead eutectic, lead bismuth eutectic or lead. When so used, plutonium-239 is consumed, and merchantable heat is produced along with fissile uranium-233, which can be denatured with uranium-238 and used in light water reactors as fuel.Type: GrantFiled: February 11, 2010Date of Patent: December 23, 2014Inventor: Charles S. Holden
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Publication number: 20140133616Abstract: A method for preparing plutonium-238 (Pu-238) using reactor may include irradiating a liquid containing a neptunium-237 (Np-237) based compounds with neutrons to convert a portion of the Np-237 based compound to a Np-238 based compound; retaining the liquid containing the resulting mixture for a sufficient amount of time for the Np-238 based compound to at least partially convert to a plutonium-238 (Pu-238) based compound. The method further may include separating the Pu-238 based compound from the neptunium based compounds using distillation or chemical method.Type: ApplicationFiled: November 13, 2012Publication date: May 15, 2014Applicant: GENERAL ATOMICSInventors: Timothy Creston BERTCH, Lloyd Chauncey BROWN
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Publication number: 20130114775Abstract: A process for producing isotopes by continuously flowing a liquid stream, carrying capsules of target nuclei (NP-237) in solution, through a nuclear reactor (a TRIGA style nuclear reactor). Upon removal from the core of the nuclear reactor and after allowing for the decay of Np-238 to Pu-238, the capsules are emptied and the mixture of elements and isotopes are chemically separated using solvent extraction or ion exchange.Type: ApplicationFiled: August 29, 2012Publication date: May 9, 2013Applicant: UNIVERSITIES SPACE RESEARCH ASSOCIATIONInventors: Steven D. HOWE, Jorge NAVARRO, Douglas CRAWFORD, Terry RING
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Publication number: 20120069946Abstract: Disclosed are a method and apparatus for making a radioisotope and a composition of matter including the radioisotope. The radioisotope is made by exposing a material to neutrons from a portable neutron source.Type: ApplicationFiled: September 22, 2010Publication date: March 22, 2012Applicant: SIEMENS MEDICAL SOLUTIONS USA, INC.Inventors: James J. Hamill, Stefan B. Siegel, Charles Russell Buchanan
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Patent number: 6896716Abstract: A method for producing ultra-pure Pu-238 is provided. The method comprises the steps of short-term irradiating Am-241 targets with a high, thermal neutron flux greater than 6.5×1014 neutrons cm?2 s?1 and more preferably greater than 1×1015 neutrons cm?2 s?1 for a predetermined period of time preferably from 20 days to 30 days and more preferably approximately 25 days to convert a substantial fraction of the Am-241 to Cm-242, e.g., approximately 0.555 g of Cm-242 per g of Am-241 charged, thereafter promptly chemically separating the produced Cm-242, preferably within 10 days to 20 days of the irradiation cycle of the Am-241 targets and more preferably within about 15 days of the irradiation cycle of the Am-241 targets, and recovering the ultra-pure Pu-238 decay product of the separated Cm-242.Type: GrantFiled: December 10, 2002Date of Patent: May 24, 2005Assignee: Haselwood Enterprises, Inc.Inventor: John E. Jones, Jr.
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Patent number: 5076971Abstract: Apparatus and method for decontaminating radioactive materials by stimulating the atomic system of radioactive materials. The stimulus is kept applied to the radioactive materials for a predetermined time. In this way, the rate of decay of the radioactivity of the materials is greatly accelerated and the materials are thereby decontaminated at a rate much faster than normal. The stimulus can be applied to the radioactive materials placing them within the sphere or terminal of a Van de Graaff generator and allowing them to be subjected to the electrical potential of the generator, such as in the range of 50 kilovolts to 500 kilovolts, for at least a period of 30 minutes or more.Type: GrantFiled: August 28, 1989Date of Patent: December 31, 1991Assignee: Altran CorporationInventor: William A. Barker
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Patent number: 4968476Abstract: A light water cooled and moderated nuclear reactor for breeding fissile material on a uranium-plutonium cycle and also a method of operating a light water cooled and moderated reactor having a prebreeder section fueled from plutonium extracted from fuel discharged by a uranium burner or converter burner core. Subsequently, the prebreeder section, together with a breeder section, operated as coupled cores or modules, becomes self-sustaining and able to breed fissile plutonium fuels at a relatively high rate of gain.Type: GrantFiled: May 14, 1982Date of Patent: November 6, 1990Assignee: Touro CollegeInventor: Alvin Radkowsky
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Patent number: 4663110Abstract: A fusion blanket includes a chamber wall, a multiplication section, an enrichment section and a reflector in radially outward succession, respectively. The chamber wall isolates the fusion reaction chamber from the remainder of the blanket. Fusion neutrons bombard atoms in the multiplication section to free further neutrons which are then available for breeding fuel. The enrichment section contains fertile fuel of sufficient dilution to maximize the enrichment rate and minimize fast fission. Materials may be included in the multiplication section and the enrichment section to reduce thermal neutron flux, thereby suppressing thermal fission. Additionally, tritium may be bred in both sections. The fertile material is exposed to neutron bombardment until the desired enrichment is achieved. The particles may be removed and mixed to minimize nonuniformities in enrichment. The particles may then be fabricated into fuel elements for fission reactors.Type: GrantFiled: May 21, 1985Date of Patent: May 5, 1987Assignee: GA Technologies Inc.Inventor: Edward T. Cheng
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Patent number: 4637900Abstract: A method is disclosed for making a fuel pellet for a nuclear reactor. A mixture is prepared of PuO.sub.2 and UO.sub.2 powders, where the mixture contains at least about 30% PuO.sub.2, and where at least about 12% of the Pu is the Pu.sup.240 isotope. To this mixture is added about 0.3 to about 5% of a binder having a melting point of at least about 250.degree. F. The mixture is pressed to form a slug and the slug is granulated. Up to about 4.7% of a lubricant having a melting point of at least about 330.degree. F. is added to the granulated slug. Both the binder and the lubricant are selected from a group consisting of polyvinyl carboxylate, polyvinyl alcohol, naturally occurring high molecular weight cellulosic polymers, chemically modified high molecular weight cellulosic polymers, and mixtures thereof. The mixture is pressed to form a pellet and the pellet is sintered.Type: GrantFiled: January 13, 1984Date of Patent: January 20, 1987Assignee: The United States of America as represented by the United States Department of EnergyInventor: James R. Frederickson
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Patent number: 4483816Abstract: A combination of passive and active neutron measurements which yields quantitative information about the isotopic composition of transuranic wastes from nuclear power or weapons material manufacture reactors is described. From the measurement of prompt and delayed neutron emission and the incidence of two coincidentally emitted neutrons from induced fission of fissile material in the sample, one can quantify .sup.233 U, .sup.235 U and .sup.239 Pu isotopes in waste samples. Passive coincidence counting, including neutron multiplicity measurement and determination of the overall passive neutron flux additionally enables the separate quantitative evaluation of spontaneous fission isotopes such as .sup.240 Pu, .sup.244 Cm and .sup.252 Cf, and the spontaneous alpha particle emitter .sup.241 Am.Type: GrantFiled: March 31, 1982Date of Patent: November 20, 1984Assignee: The United States of America as represented by the Department of EnergyInventors: John T. Caldwell, Walter E. Kunz, James D. Atencio